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High Entropy Wide Bandgap Borates with Broadband Luminescence and Strong Nonlinear Optical Properties
The IRG team has discovered new high-entropy rare earth borate (RnBBO) single crystals with compositions R5Ba3(B3O6)3 and R6Ba3(B3O6)3 (R = Nd, Tb, Sm, Dy, Gd, Yb, Er). These systems have been grown in the form of large single crystals with bandgaps > 5 eV, enhanced optical transparency, broadband luminescence spanning IR to UV wavelengths, and very high laser damage thresholds.
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Orbital Hybridization-Induced Ising-Type Superconductivity in a Confined Gallium Layer
The coupling between an electron’s orbital motion and its spin can give rise to unconventional superconducting states where the pairing between the electrons that creates the superconductivity has an Ising-like character, meaning that the spins are “locked” to be perpendicular to the 2D layer.
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Room-temperature charge localization in ion-coupled bilayer transistors
The ability to localize mobile charges in solids is essential for understanding a range of correlated electron transport phenomena. Yet, existing approaches rely on weak interaction potentials, limiting their applicability to low-temperature conditions. Park, Liu and Vaikuntanathan addressed this challenge by creating ion-gated bilayer transistors based on hybrid bilayer crystals, composed of a monolayer perylene diimide molecular crystal stacked on a monolayer of molybdenum disulfide.
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Suspensions of Particles with Tunable Shape Memory
A 3-way collaboration between the de Pablo, Rowan and Jaeger groups in IRG 1 developed a novel class of suspensions with tunable memory. The particles are made from liquid crystalline elastomers (LCEs) and exhibit anisotropic elasticity and shape-shifting characteristics. In these suspensions small changes in temperature can be used to induce large changes in material stiffness and transform the particle shape, thereby providing access to a wide range of different flow behaviors. In particular, ajammed, non-flowing state can be escaped by activating the shape memory behavior if the LCE particle.
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Mapping the Landscape of Topological Magnons: From High-Throughput Discovery to Experimental Realization
The MRSEC team at Ohio State University developed and applied a fully automated algorithm to screen all 1,649 known magnetically ordered materials, identifying 387 (~23%) as candidates guaranteed to host topological magnons when a magnetic field, electric field, or strain is applied — a >30× expansion of the known candidate pool.
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Strain Control of Structure and Emergent Magnetism in LaCoO3 Thin Films
Strain engineering in epitaxial LaCoO3 thin films enables direct control of crystal symmetry and spin state population, revealing a clear pathway from lattice distortion to emergent magnetism in correlated oxides.
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Quantum Sensing of Broadband Spin Dynamics and Magnon Transport in Antiferromagnets
Quantum sensing enables spatially localized, broadband detection of spin dynamics and magnon transport in antiferromagnets, addressing a key limitation of conventional magnetic resonance techniques.
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Electrostatic Complexes of Conjugated Polyelectrolytes for Printable Electronics
Conjugated polyelectrolytes can be used to form biosensors and bioelectronic devices. Controlling the optoelectronic properties of conjugated polyelectrolytes typically requires extensive synthetic modification.
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Fast Phase Prediction of Charged Polymer Blends by White-Box Machine Learning Surrogates
Previously, UC Santa Barbara MRSEC researchers demonstrated that the introduction of charge to typically immiscible polymer blends can induce a microphase separation. Based on that work, the Random Phase Approximation (RPA) can be used with 13 input parameters to determine if a blend is microphase separated or homogeneous.
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Superlubricious Hydrogels from Oxidation Gradients
Hydrogels are hydrated three-dimensional networksof hydrophilic polymers that are commonly used in the biomedical industry due to their mechanical and structural tunability, biocompatibility, and similar water content to biological tissues.
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